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Tetrafluoroborate (dicarbonylmethylidine-cyclotris ((cyclopentadienyl) rhodium))

Tetrafluoroborate [dicarbonylmethylidine-cyclotris [(cyclopentadienyl) rhodium}] is the carbonyl complex of the organometallic rhodium and cyclopentadiene of the composition [Rh 3 (C 5 H 5 ) 3 (CH) (CO) 2 ] [BF 4 ], black crystals.

Tetrafluoroborate [dicarbonylmethylidine-cyclotris {(cyclopentadienyl) rhodium}]
Are common
Systematic
name
Tetrafluoroborate [dicarbonylmethylidine-cyclotris {(cyclopentadienyl) rhodium}]
Traditional namesTetrafluoroborate [μ-dicarbonyl-μ 3 -methylidine- cyclo- tris {(η-cyclopentadienyl) rhodium}]
Chem. formula[Rh 3 (C 5 H 5 ) 3 (CH) (CO) 2 ] [BF 4 ]
Rat formula[Rh 3 (η-C 5 H 5 ) 3 (μ 3 -CH) (μ-CO) 2 ] [BF 4 ]
Physical properties
conditionblack crystals
Molar mass659.84 g / mol
Thermal properties
T. decomp.> 280 ° C

Getting

  • An aqueous solution of hydrogen tetrafluoroborate is added to a solution of methylenebis [carbonyl (cyclopentadienyl) rhodium] in tetrahydrofuran :
3CH2[Rh(CfiveHfive)(CO)]2+H[BFfour]→{\ displaystyle {\ mathsf {3CH_ {2} [Rh (C_ {5} H_ {5}) (CO)] _ {2} + H [BF_ {4}] \ {\ xrightarrow {}} \}}}  
→80oC2[Rh3(CfiveHfive)3(CH)(CO)2][BFfour]+2CO+CHfour+H2{\ displaystyle {\ mathsf {\ {\ xrightarrow {80 ^ {o} C}} \ 2 [Rh_ {3} (C_ {5} H_ {5}) _ {3} (CH) (CO) _ {2 }] [BF_ {4}] + 2CO + CH_ {4} + H_ {2}}}}  

Physical Properties

Tetrafluoroborate [dicarbonylmethylidine-cyclotris {(cyclopentadienyl) rhodium}] forms black crystals of monoclinic syngony , space group C 2 / c .

Stable in air, soluble in acetonitrile, acetone and methanol, insoluble in tetrahydrofuran , methylene dichloride , diethyl ether and aliphatic hydrocarbons .

Literature

  • Inorganic Synthesis Guide: 6 Vol. / Ed. Brower G. - M .: Mir, 1986 .-- T. 6 .-- 360 p.


Source - https://ru.wikipedia.org/w/index.php?title= Tetrafluoroborate_ ( dicarbonyl - methylidine - cyclo- tris( ( cyclopentadienyl)rodium :))& oldid = 81003220


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